Morphology, Microstructure, and Rheology of Amphiphilic Telechelics Incorporating Polyhedral Oligosilsesquioxane

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Morphology, Microstructure, and Rheology of Amphiphilic Telechelics Incorporating Polyhedral Oligosilsesquioxane

Amphiphilic telechelics incorporating polyhedral oligosilsesquioxane (POSS) end-caps were synthesized and studied as a novel building block for the construction of inorganic-organic hybrid materials. Their micron-scale morphologies were investigated using hot-stage polarizing optical microscopy (POM), revealing a dramatic influence of POSS macromer incorporation. The molecular-scale crystalline...

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Biodegradable thermoplastic polyurethanes incorporating polyhedral oligosilsesquioxane.

A new hybrid thermoplastic polyurethane (TPU) system that incorporates an organic, biodegradable poly(D, L-lactide) soft block with a hard block bearing the inorganic polyhedral oligosilsesquioxane (POSS) moiety is introduced and studied. Changes in the polyol composition made through variation of the hydrophilic initiator molecular weight show direct control of the final transition temperature...

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Rheological Behavior of Entangled Polystyrene - Polyhedral Oligosilsesquioxane ( POSS ) Copolymer (

We report on the linear viscoelastic properties of a family of entangled linear thermoplastic nonpolar hybrid inorganic-organic polymers: random copolymers of polystyrene (PS) and styryl-based polyhedral oligosilsesquioxane (POSS), R7(Si8O12)(C6H4CHdCH2), with R ) isobutyl (iBu). A series of styrene-styryl POSS random copolymers with 0, 6, 15, 30, and 50 wt % iBuPOSS were investigated. WAXS and...

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Rheological Behavior of Entangled Polystyrene-Polyhedral Oligosilsesquioxane (POSS) Copolymers

We report on the linear viscoelastic properties of a family of entangled linear thermoplastic nonpolar hybrid inorganic-organic polymers: random copolymers of polystyrene (PS) and styryl-based polyhedral oligosilsesquioxane (POSS), R7(Si8O12)(C6H4CHdCH2), with R ) isobutyl (iBu). A series of styrene-styryl POSS random copolymers with 0, 6, 15, 30, and 50 wt % iBuPOSS were investigated. WAXS and...

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Rheological Behavior of Entangled Polystyrene - Polyhedral Oligosilsesquioxane ( POSS )

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ژورنال

عنوان ژورنال: Macromolecules

سال: 2006

ISSN: 0024-9297,1520-5835

DOI: 10.1021/ma062069i